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This has been my experience for 4* magicite too. The drops don't seem to be weighted evenly, the primary boss magicite seems to drop 9:1 for the others.
Had 8 isgebind in a row. Took an eternity to get 3x dullahan. Similar with Marilis and Midgarsormr. Saw a ton of those, the others, not so much.
RNG. I was looking for Midgardsomr yesterday and it took about 12 S/Ls to get one. Kept getting Earth Guardian and Catastrophe, to the point where I started to wonder if "Midgardsomr" had been renamed to "Earth Guardian" in Kompanion (I never checked out Midgardsomr's 4* drops before).
ShinUltima - The Right Arm of Scrub Voltron PSN: ShinUltima